The far-wing line shape theory within the binary collision and
quasistatic framework has been developed using the coordinate
representation. Within this formalism, the main computational task
is the evaluation of multidimensional integrals whose variables are
the orientational angles needed to specify the initial and final
positions of the system during transition processes. Using standard
methods, one is able to evaluate the 7-dimensional integrations
required for linear molecular systems, or the 7-dimensional
integrations for more complicated asymmetric-top (or symmetric-top)
molecular systems whose interaction potential contains cyclic
coordinates. In order to obviate this latter restriction on the
form of the interaction potential, a Monte Carlo method is used to
evaluate the 9-dimensional integrations required for systems
consisting of one asymmetric-top (or symmetric-top) and one linear
molecule, such as H20-N2. Combined with techniques developed
previously to deal with sophisticated potential models, one is able
to implement realistic potentials for these systems and derive
accurate, converged results for the far-wing line shapes and the
corresponding absorption coefficients. Conversely, comparison of
the far-wing absorption with experimental data can serve as a
sensitive diagnostic tool in order to obtain detailed information
on the short-range anisotropic dependence of interaction
potentials.
General
| Imprint: |
Bibliogov
|
| Country of origin: |
United States |
| Release date: |
August 2013 |
| First published: |
August 2013 |
| Authors: |
Q. Ma
|
| Dimensions: |
246 x 189 x 2mm (L x W x T) |
| Format: |
Paperback - Trade
|
| Pages: |
38 |
| ISBN-13: |
978-1-289-28248-6 |
| Categories: |
Books >
Social sciences >
Politics & government >
General
Promotions
|
| LSN: |
1-289-28248-X |
| Barcode: |
9781289282486 |
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