various places of the world. Thus, it is hoped that this up-to-date subseries would increase the "awareness" of the world's citizens and encourage governments to devote more attention and resources to address this issue. The series editors thank the international panel of contributors for bringing this timely series into completion. We also wish to acknowledge the very insightful input of the following colleagues: Prof. A. L. Page ofthe University of California, Prof. T. C. Hutchinson of the University of Toronto, and Dr. Steve Lindberg of the Oak Ridge National Laboratory. We also wish to thank the superb effort and cooperation of the volume editors in handling their respective volumes. The constructive criticisms of chapter reviewers also deserve much appreciation. Finally, we wish to convey our appreciation to my secretary, Ms. Brenda Rosier, and my technician, Ms. Claire Carlson, for their very able assistance in various aspects of this series. Aiken, South Carolina Domy C. Adriano Coordinating Editor Preface to Acidic Precipitation, Volume 4 (Advances in Environmental Science) Acidic precipitation and its effects have been the focus ofintense research for over two decades. Initially, research centered on the acidity status and acidification of surface waters and consequent impact on the status of sports fisheries; evidence suggested impacts on fisheries in Sweden and Norway, and in North America, in eastern Ontario, Quebec, and in the Adirondack Mountains of New York.

countries accelerating to reach a consensus on the role that atmospheric emissions and acidic precipitation play in the environment, publication of this series is timely. The editors thank the contributors to this volume for their efforts in describing a wide array of atmospheric topics, all of which are important to an understanding of the acidic precipitation issue. Oak Ridge, Tennessee Steven E Lindberg Riverside, California Albert L. Page Orono, Maine Stephen A. Norton Contents Series Preface .................................................... v Preface... ....... ...... ..... ... .. ............................... .. vii Contributors ..................................................... xiii Sources of Acids, Bases, and Their Precursors in the Atmosphere . . . 1 Roger L. Tanner I. Introduction and Definitions. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 1 II. Sources of Acids ............................................... 3 III. Sources of Acid-Neutralizing Substances (Bases) ................... 9 IV. Distribution of Atmospheric Acids and Bases ...................... 10 V. Gas-Aerosol Equilibria and Boundary Layer Mixing ................ 14 VI. Summary of Significant Acid-Formation Pathways.............. . .. . 15 References ................................ ................... 17 Aerosol Sulfur Association with Aluminum in Eastern North America: Evidence for Solubilization of Atmospheric Trace Metals before Deposition ......... . . . . . . . . . . 21 . . ."

countries accelerating to reach a consensus on the role that atmospheric emissions and acidic precipitation play in the environment, publication of this series is timely. The editors thank the contributors to this volume for their efforts in describing a wide array of atmospheric topics, all of which are important to an understanding of the acidic precipitation issue. Oak Ridge, Tennessee Steven E Lindberg Riverside, California Albert L. Page Orono, Maine Stephen A. Norton Contents Series Preface .................................................... v Preface... ....... ...... ..... ... .. ............................... .. vii Contributors ..................................................... xiii Sources of Acids, Bases, and Their Precursors in the Atmosphere . . . 1 Roger L. Tanner I. Introduction and Definitions. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 1 II. Sources of Acids ............................................... 3 III. Sources of Acid-Neutralizing Substances (Bases) ................... 9 IV. Distribution of Atmospheric Acids and Bases ...................... 10 V. Gas-Aerosol Equilibria and Boundary Layer Mixing ................ 14 VI. Summary of Significant Acid-Formation Pathways.............. . .. . 15 References ................................*................... 17 Aerosol Sulfur Association with Aluminum in Eastern North America: Evidence for Solubilization of Atmospheric Trace Metals before Deposition ......... . . . . . . . . . . 21 . . .

various places of the world. Thus, it is hoped that this up-to-date subseries would increase the "awareness" of the world's citizens and encourage governments to devote more attention and resources to address this issue. The series editors thank the international panel of contributors for bringing this timely series into completion. We also wish to acknowledge the very insightful input of the following colleagues: Prof. A. L. Page ofthe University of California, Prof. T. C. Hutchinson of the University of Toronto, and Dr. Steve Lindberg of the Oak Ridge National Laboratory. We also wish to thank the superb effort and cooperation of the volume editors in handling their respective volumes. The constructive criticisms of chapter reviewers also deserve much appreciation. Finally, we wish to convey our appreciation to my secretary, Ms. Brenda Rosier, and my technician, Ms. Claire Carlson, for their very able assistance in various aspects of this series. Aiken, South Carolina Domy C. Adriano Coordinating Editor Preface to Acidic Precipitation, Volume 4 (Advances in Environmental Science) Acidic precipitation and its effects have been the focus ofintense research for over two decades. Initially, research centered on the acidity status and acidification of surface waters and consequent impact on the status of sports fisheries; evidence suggested impacts on fisheries in Sweden and Norway, and in North America, in eastern Ontario, Quebec, and in the Adirondack Mountains of New York.