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This graduate text gives an introductory overview of the fundamentals of quantum nonlinear optics. It deals with the organization of radiation field, interaction between electronic system and radiation field, statistics of light, mutual manipulation of light and matter, laser oscillation, dynamics of light, nonlinear optical response, nonlinear spectroscopy as well as ultrashort and ultrastrong laser pulse. In addition, latest results of the frontier of this science are presented. Problems and solutions help the reader to become familiar with the material given.
An exciton is an electronic excitation wave consisting of an electron-hole pair which propagates in a nonmetallic solid. Since the pioneering research of Fren kel, Wannier and the Pohl group in the 1930s, a large number of experimental and theoretical studies have been made. Due to these investigations the exciton is now a well-established concept and the electronic structure has been clarified in great detail. The next subjects for investigation are, naturally, dynamical processes of excitons such as excitation, relaxation, annihilation and molecule formation and, in fact, many interesting phenomena have been disclosed by recent works. These excitonic processes have been recognized to be quite important in solid-state physics because they involve a number of basic interactions between excitons and other elementary excitations. It is the aim of this quasi monograph to describe these excitonic processes from both theoretical and experimental points of view. we take a few To discuss and illustrate the excitonic processes in solids, important and well-investigated insulating crystals as playgrounds for excitons on which they play in a manner characteristic of each material. The selection of the materials is made in such a way that they possess some unique properties of excitonic processes and are adequate to cover important interactions in which excitons are involved. In each material, excitonic processes are described in detail from the experimental side in order to show the whole story of excitons in a particular material."
This is the Proceedings of the Taniguchi International Symposium on "Relaxation of Elementary Excitations" which was held October 12-16,1979, at Susono-shi (at the foot of f1t. Fuji) in Japan. The pleasant atmosphere of the Symposium is evidenced in the picture of the participants shown on the next page. The purpose of the symposium was to provide an opportunity for a limited number of active researchers to meet and to discuss relaxation processes and related phenomena not only of excitons and phonons in solids but also electronic and vibrational excitations in molecules and biological systems. First, the lattice relaxation, i.e., multi-phonon process, associated with electronic excitation, which plays important roles in self-trapping of an exciton and a particle (electron and hole) and also in degradation of semi conductor lasers, is discussed. Second, this lattice relaxation is studied as the intermediate state interaction in the second-order optical responses, i.e., in connection with the competitive behavior of Raman scattering and luminescence. Third, relaxation mechanisms and relaxation constants are by spectroscopic methods as well as by genuine nonlinear optical determined phenomena. Conversely the relaxation is decisive in coherent nonlinear optical phenomena such as laser, superradiance, and optical bistability. Fourth, the role played by relaxation processes is discussed for optical phenomena in macromolecules and biological system such as photosynthesis."
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