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This book summarizes several years of research carried out by a
collaboration of many groups on ultrafast photochemical reactions.
It emphasizes the analysis and characterization of the nuclear
dynamics within molecular systems in various environments induced
by optical excitations and the study of the resulting molecular
dynamics by further interaction with an optical field.
The present monograph summarizes, in a comprehensive way,
several years of joint experimental and theoretical frontier
research on ultrafast laser-induced molecular dynamics and its
control. Emphasis is set on the characterization of the nuclear
dynamics within molecular systems in various environments (gas
phase, surfaces, solids, solution, strong fields) triggered by
optical excitations spanning from the infrared to the ultraviolet.
Building on the converged analysis between experiment and theory,
control of chemical reactions is established by means of optimally
shaped laser pulses. This paves the road toward new applications
and future challenges in this rapidly developing research
field.
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