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This thesis introduces a series of novel, non-conjugated
polyarylether hosts that are not subject to the triplet-energy
limitations of traditional conjugated polymer hosts. As a result of
this major breakthrough, the long-standing problem of triplet
energy back transfer has now been overcome, making it possible to
design high-efficiency electrophosphorescent polymers (PhPs),
especially the blue and all-phosphorescent white ones. In addition,
the author proposes a spiro-linked hyperbranched architecture for
PhPs to inhibit the undesired triplet energy back transfer process
in low triplet-energy hosts. The work in this thesis provides vital
new insights into the design of PhPs and has led to several
publications in high-profile journals.
This thesis introduces a series of novel, non-conjugated
polyarylether hosts that are not subject to the triplet-energy
limitations of traditional conjugated polymer hosts. As a result of
this major breakthrough, the long-standing problem of triplet
energy back transfer has now been overcome, making it possible to
design high-efficiency electrophosphorescent polymers (PhPs),
especially the blue and all-phosphorescent white ones. In addition,
the author proposes a spiro-linked hyperbranched architecture for
PhPs to inhibit the undesired triplet energy back transfer process
in low triplet-energy hosts. The work in this thesis provides vital
new insights into the design of PhPs and has led to several
publications in high-profile journals.
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