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This thesis experimentally demonstrates the much discussed
electronic charge-glass states in solids. It focuses on
quasi-two-dimensional organic conductors of the -(BEDT-TTF)2X
family, which form anisotropic triangular lattices, and examines
their electronic properties using various measurements:
resistivity, time-resolved electric transport, X-ray diffraction
analysis, and nuclear magnetic resonance spectroscopy. The hallmark
of the charge glass caused by geometrical frustration of lattice
structure for those materials is successfully observed for the
first time. The thesis provides new insights into the exotic
properties of matter driven by strong electron correlations and
crystalline frustration. The introduction enables beginners to
understand fundamentals of the charge-glass states and the
organic-conductor family -(BEDT-TTF)2X. The comprehensive and
detailed descriptions of the experimental demonstration make this a
valuable resource.
This thesis experimentally demonstrates the much discussed
electronic charge-glass states in solids. It focuses on
quasi-two-dimensional organic conductors of the -(BEDT-TTF)2X
family, which form anisotropic triangular lattices, and examines
their electronic properties using various measurements:
resistivity, time-resolved electric transport, X-ray diffraction
analysis, and nuclear magnetic resonance spectroscopy. The hallmark
of the charge glass caused by geometrical frustration of lattice
structure for those materials is successfully observed for the
first time. The thesis provides new insights into the exotic
properties of matter driven by strong electron correlations and
crystalline frustration. The introduction enables beginners to
understand fundamentals of the charge-glass states and the
organic-conductor family -(BEDT-TTF)2X. The comprehensive and
detailed descriptions of the experimental demonstration make this a
valuable resource.
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