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Simulation Studies of Recombination Kinetics and Spin Dynamics in Radiation Chemistry (Paperback, Softcover reprint of the original 1st ed. 2014)
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Simulation Studies of Recombination Kinetics and Spin Dynamics in Radiation Chemistry (Paperback, Softcover reprint of the original 1st ed. 2014)
Series: Springer Theses
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Amit Agarwal’s thesis reports a substantial contribution to the
microscopic simulation of radiation chemical reactions. In his
research Agarwal extends existing models to further understand
scavenging, spin and relaxation effects. This research has
advanced the development of both the Monte Carlo Random Flights and
the Independent Reaction Times (IRT) simulation
tools. Particular highlights are the extension of these tools
to include both the spin-exchange interaction and spin relaxation,
both of which are influential in radiolytic systems where many
reactions are spin-controlled. In addition, the study has led
to the discovery of a novel correlation of the scavenging rate with
the recombination time in low permittivity solvents. This finding
goes against existing assumptions underlying the theory of
diffusion kinetics while still being accommodated in the IRT method
which demonstrates the power of this unconventional approach. The
work in this thesis can be applied to a wide number of fields
including the nuclear industry, medicine, food treatment,
polymer curing, the preparation of nano-colloids, power generation
and waste disposal.
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