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Simulation Studies of Recombination Kinetics and Spin Dynamics in Radiation Chemistry (Hardcover, 2014 ed.)
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Simulation Studies of Recombination Kinetics and Spin Dynamics in Radiation Chemistry (Hardcover, 2014 ed.)
Series: Springer Theses
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Total price: R3,690
Discovery Miles: 36 900
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Amit Agarwal's thesis reports a substantial contribution to the
microscopic simulation of radiation chemical reactions. In his
research Agarwal extends existing models to further understand
scavenging, spin and relaxation effects. This research has advanced
the development of both the Monte Carlo Random Flights and the
Independent Reaction Times (IRT) simulation tools. Particular
highlights are the extension of these tools to include both the
spin-exchange interaction and spin relaxation, both of which are
influential in radiolytic systems where many reactions are
spin-controlled. In addition, the study has led to the discovery of
a novel correlation of the scavenging rate with the recombination
time in low permittivity solvents. This finding goes against
existing assumptions underlying the theory of diffusion kinetics
while still being accommodated in the IRT method which demonstrates
the power of this unconventional approach. The work in this thesis
can be applied to a wide number of fields including the nuclear
industry, medicine, food treatment, polymer curing, the preparation
of nano-colloids, power generation and waste disposal.
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