This thesis addresses the introduction of redox mediator into
lithium-oxygen batteries to improve their electrochemical
performance especially in terms of practical energy density and
round-trip efficiency. In chapter 1, basic electrochemistry
regarding lithium-oxygen batteries and redox mediators are
introduced. In chapter 2 to 4, comprehensive researches including
the discovery of a new redox mediator inspired by biological
system, the investigation on kinetic property of redox mediator,
and the prevention of shuttle phenomenon are introduced, followed
by chapter 5 summarizing the contents. This thesis is targeted to
students and researchers interested in electrochemistry and energy
storage systems.
General
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