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In this thesis, the author describes the total synthesis of natural
product Maoecrystal V in detail. In the first part of the thesis,
the author introduces the research background and reviews the
research progress in total synthesis of Maoecrystal V. In the
second part, the author develops a novel and concise approach for
the stereo selective construction of the tetracyclic model system
of Maoecrystal V. The model system is accomplished in 8 steps with
20% yield. In the third part, the author describes the first
successful total synthesis of Maoecrystal V and investigates four
strategies for constructing the key tetrahydrofuran oxa-bridge
skeleton. The total synthesis starts from a known compound and is
accomplished in 17 steps with 1.2% yield. The successful total
synthesis of Maoecrystal V will contribute to the development of
efficient synthetic strategies for natural products and other
compounds with complex structures.
In this thesis, the author describes the total synthesis of
natural product Maoecrystal V in detail. In the first part of the
thesis, the author introduces the research background and reviews
the research progress in total synthesis of Maoecrystal V. In the
second part, the author develops a novel and concise approach for
the stereo selective construction of the tetracyclic model system
of Maoecrystal V. The model system is accomplished in 8 steps with
20% yield. In the third part, the author describes the first
successful total synthesis of Maoecrystal V and investigates four
strategies for constructing the key tetrahydrofuran oxa-bridge
skeleton. The total synthesis starts from a known compound and is
accomplished in 17 steps with 1.2% yield. The successful total
synthesis of Maoecrystal V will contribute to the development of
efficient synthetic strategies for natural products and other
compounds with complex structures.
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