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Heterocyclic Carbene Complexes (Paperback)
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Heterocyclic Carbene Complexes (Paperback)
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N-heterocyclic carbenes have become established as efficient
ancillary ligands for homogeneous catalysis, and an increasing
number of catalytic transformations have been carried out using
transition-metal carbene complexes. This book describes the
synthesis of a broad range of heterocyclic carbene complexes of
transition metals, their fundamental reaction chemistry and their
use as catalysts in a number of reactions. Mechanistic studies have
been performed in order to gain insight into likely catalytic
cycles and the decomposition processes of the complexes. The
reductive elimination of carbenes with alkyl, aryl, acyl and
hydride groups to give the imidazolium cation was discovered, and
it was demonstrated that this reaction represents a serious mode to
catalyst deactivation for late transition metals. Some strategies
to alleviate this effect have been identified, resulting in the
development of highly active catalysts for a number of reactions.
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