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Light Scattering From Micrometric Mineral Dust and Aggregate Particles - Effects of Structure and Shape Applied to Paleoclimate Studies (Hardcover, 1st ed. 2020)
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Light Scattering From Micrometric Mineral Dust and Aggregate Particles - Effects of Structure and Shape Applied to Paleoclimate Studies (Hardcover, 1st ed. 2020)
Series: Springer Theses
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Light scattering from particles in the nanometric and micrometric
size range is relevant in several research fields, such as aerosol
science and nanotechnology. In many applications, the description
of the optical properties of non-spherical, inhomogeneous particles
is still inadequate or requires demanding numerical calculations.
Lorenz-Mie scattering and effective medium approximations represent
currently the main theoretical tools to model such particles, but
their effectiveness has been recently called into question. This
work examines how the morphology of a particle affects its
scattering parameters from an experimental standpoint, supporting
findings with extensive simulations. The dust content of Antarctic,
Greenlandic, and Alpine ice cores is analysed with a
particle-by-particle approach. Moreover, a study on colloidal
aggregates shows that correlations among the fields radiated by
primary particles are responsible for the poor agreement of
effective medium approximations with experimental results. On the
theoretical side, an interpretation in terms of the structure
factor is given, which satisfactorily describes the data. The
insights of this thesis are relevant for quantifying the
contribution of mineral dust to the radiative energy balance of the
Earth.
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