Ruthenium compounds have shown very good second order and third
order behaviour. Very high non-linear optical (NLO) response is due
to the extensive coordination and organometallic chemistry of
ruthenium. Electron-rich d6 ruthenium (II) centres are especially
well-suited for incorporation into NLO chromophores because their
highly polarizable d orbitals can cause effective
-electron-donating properties when coordinated to ligands with
low-lying * orbitals. This work provides an understanding of the
NLO properties of ruthenium complexes. All systems display large
second-order NLO response. This effort may provide the guidelines
to synthesize the high-performance NLO materials. The present
investigation gives insight into the NLO response of ruthenium
complexes and endeavors to disclose the origin of the NLO response
of this family, which is interesting and important in design and
synthesis of new promising NLO materials."
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