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Emergent States in Photoinduced Charge-Density-Wave Transitions (Hardcover, 1st ed. 2021)
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Emergent States in Photoinduced Charge-Density-Wave Transitions (Hardcover, 1st ed. 2021)
Series: Springer Theses
Expected to ship within 12 - 17 working days
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This book advances understanding of light-induced phase transitions
and nonequilibrium orders that occur in a broken-symmetry system.
Upon excitation with an intense laser pulse, materials can undergo
a nonthermal transition through pathways different from those in
equilibrium. The mechanism underlying these photoinduced phase
transitions has long been researched, but many details in this
ultrafast, non-adiabatic regime still remain to be clarified. The
work in this book reveals new insights into this phenomena via
investigation of photoinduced melting and recovery of charge
density waves (CDWs). Using several time-resolved diffraction and
spectroscopic techniques, the author shows that the light-induced
melting of a CDW is characterized by dynamical slowing-down, while
the restoration of the symmetry-breaking order features two
distinct timescales: A fast recovery of the CDW amplitude is
followed by a slower re-establishment of phase coherence, the
latter of which is dictated by the presence of topological defects
in the CDW. Furthermore, after the suppression of the original CDW
by photoexcitation, a different, competing CDW transiently emerges,
illustrating how a hidden order in equilibrium can be unleashed by
a laser pulse. These insights into CDW systems may be carried over
to other broken-symmetry states, such as superconductivity and
magnetic ordering, bringing us one step closer towards manipulating
phases of matter using a laser pulse.
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