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Theory of Nonlinear Propagation of High Harmonics Generated in a Gaseous Medium (Hardcover, 2013 ed.)
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Theory of Nonlinear Propagation of High Harmonics Generated in a Gaseous Medium (Hardcover, 2013 ed.)
Series: Springer Theses
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Theory of Nonlinear Propagation of High Harmonics Generated in a
Gaseous Medium establishes the theoretical tools to study
High-Order Harmonic Generation (HHG) by intense ultrafast infrared
lasers in atoms and molecules. The macroscopic propagation of both
laser and high-harmonic fields is taken into account by solving
Maxwell's wave equations, while the single-atom or single-molecule
response is treated with a quantitative rescattering theory by
solving the time-dependent Schroedinger equation. This book
demonstrates for the first time that observed experimental HHG
spectra of atoms and molecules can be accurately reproduced
theoretically when precise experimental conditions are known. The
macroscopic HHG can be expressed as a product of a macroscopic wave
packet and a photorecombination cross section, where the former
depends on laser and experimental conditions while the latter is
the property of target atoms or molecules. The factorization makes
it possible to retrieve microscopically atomic or molecular
structure information from the measured macroscopic HHG spectra.
This book also investigates other important issues about HHG, such
as contributions from multiple molecular orbitals, the minimum in
the HHG spectrum, the spatial mode of laser beams, and the
generation of an isolated attosecond pulse. Additionally, this book
presents the photoelectron angular distribution of aligned
molecules ionized by the HHG light.
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