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The Siamese-Twin Porphyrin and Its Copper and Nickel Complexes: A Non-Innocent Twist (Hardcover, 2014 ed.)
Loot Price: R3,737
Discovery Miles 37 370
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The Siamese-Twin Porphyrin and Its Copper and Nickel Complexes: A Non-Innocent Twist (Hardcover, 2014 ed.)
Series: Springer Theses
Expected to ship within 10 - 15 working days
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This thesis describes the first and long-sought successful
synthesis of a new pyrazole-expanded porphyrin, a higher analog of
porphyrin. This "Siamese-Twin Porphyrin" provides two conjoined
porphyrin-like coordination spheres, thus being able to accommodate
two metal ions within the same ligand. In her thesis, Lina Blusch
not only explains the challenging synthesis and characterization of
the ligand system, but also its application to the synthesis of
homo- and hetero-bimetallic Ni and Cu complexes. She observes
interesting metal-metal-interactions in the complexes, that lead to
a non-innocent multistep redox chemistry. The ligand system and its
complexes show an intriguing twisted geometry, giving rise to
helical chirality and other fascinating properties. This study
explores the first steps and opens up a new chemistry of expanded
porphyrins with the potential to biomimetic applications.
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