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Heterogenous Photochemical Electron Transfer (Hardcover)
Loot Price: R2,882
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Heterogenous Photochemical Electron Transfer (Hardcover)
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The present monograph attempts to unify these diverse and exciting
new developments within a common framework. First, the physical
principles underlying heterogenous electron-transfer processes are
outlined in a concise way and are compared to the homogeneous
counterpart. This analysis includes the notion of the Fermi level
in liquids and solids as well as the distribution of electronic
energy levels in solids and liquids. A comparison is made between
the salient kinetic features of homogeneous and heterogeneous
electron transfer reactions. This establishes the basis for the
subsequent treatment of the transduction of excitation energy and
photo-initiated electron transfer in organized molecular
assemblies, such as micelles, vesicles and monolayers.
Transmembrane redox processes are critically reviewed. Particular
attention is given to semiconductor electrodes and particles. This
includes a discussion of quantum size effects, the nature of space
charge layers as well as surface states and the dynamics of charge
carrier-induced redox reactions at the semiconductor solution
interface. These processes are of fundamental importance in such
diverse fields as photochromism, electrochromic displays,
electroreprography and photography, information storage,
photocatalysis, photodegradation of paints, and solar energy
conversion.
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