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Resolving Strong Field Dynamics in Cation States of CO_2 via Optimised Molecular Alignment (Hardcover, 2014)
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Resolving Strong Field Dynamics in Cation States of CO_2 via Optimised Molecular Alignment (Hardcover, 2014)
Series: Springer Theses
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This thesis presents an experimental study of the ultrafast
molecular dynamics of CO_2 DEGREES+ that are induced by a strong,
near-infrared, femtosecond laser pulse. In particular, typical
strong field phenomena such as tunneling ionisation, nonsequential
double ionisation and photo-induced dissociation are investigated
and controlled by employing an experimental technique called
impulsive molecular alignment. Here, a first laser pulse fixes the
molecule in space, such that the molecular dynamics can be studied
as a function of the molecular geometry with a second laser pulse.
The experiments are placed within the context of the study and
control of ultrafast molecular dynamics, where sub-femtosecond (10
DEGREES-15 seconds) resolution in ever larger molecular systems
represents the current frontier of research. The thesis presents
the required background in strong field and molecular physics,
femtosecond laser architecture and experimental techniques in a
clear and accessible language that does not require any previous
knowledge in
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