Polaritonic chemistry is an emergent interdisciplinary field in
which the strong interaction of organic molecules with confined
electromagnetic field modes is exploited in order to manipulate the
chemical structure and reactions of the system. In the regime of
strong light-matter coupling the interaction with the
electromagnetic vacuum obliges us to redefine the concept of a
molecule and consider the hybrid system as a whole. This thesis
builds on the foundations of chemistry and quantum electrodynamics
in order to provide a theoretical framework to describe these
organic light-matter hybrids. By fully embracing the structural
complexity of molecules, this theory allows us to employ
long-established quantum chemistry methods to understand
polaritonic chemistry. This leads to predictions of substantial
structural changes in organic molecules and the possibility of
significantly influencing chemical reactions both in the excited
and ground states of the system.
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