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Books > Science & Mathematics > Physics > States of matter > Condensed matter physics (liquids & solids)
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Orthogonal Supramolecular Interaction Motifs for Functional Monolayer Architectures (Hardcover, 2012 ed.)
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Orthogonal Supramolecular Interaction Motifs for Functional Monolayer Architectures (Hardcover, 2012 ed.)
Series: Springer Theses
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Deniz Yilmaz' thesis describes a combination of orthogonal
supramolecular interactions for the design of functional monolayer
architectures on surfaces, that can be used as chemical and
biosensors in a wide range of applications. The term "orthogonal
supramolecular interactions" refers to non-covalent interactions
that do not influence each other's assembly properties. Orthogonal
self-assembly thus allows extended control over the self-assembly
process and promotes new materials properties. The first part of
the thesis employs orthogonal host-guest and lanthanide-ligand
coordination interaction motifs to create supramolecular
luminescent monolayers. The second part of the thesis describes the
fabrication of functional monolayers on silicon and gold substrates
for applications in electronics. The results illustrate the power
of weak supramolecular interactions to direct the immobilization of
functional systems on surfaces. The combination of host-guest and
lanthanide-ligand coordination interaction motifs on surfaces
demonstrates that hybrid, multifunctional supramolecular monolayers
can be fabricated by integrating different non-covalent
interactions in the same system. This combination opens up new
avenues for the fabrication of complex hybrid organic-inorganic
materials and stimuli-responsive surfaces. Their utility is
demonstrated through applications of the functional interfaces to
biosensing and nanotechnology.
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