This thesis describes longitudinal nuclear relaxation measurements
of solid 129Xe near 77 K with previously unattainable
reproducibility, and demonstrates differences in relaxation,
dependent upon the way in which the solid is condensed. These
results are directly applicable to the generation and storage of
large quantities of hyperpolarized 129Xe for various applications,
such as lung magnetic resonance imaging (MRI). The thesis features
a sophisticated theoretical approach to these data sets, including
modifications to a well-established Raman-phonon scattering theory
that may explain the larger scatter in and discrepancies with
previous work.
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