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Imaging Light with Photoelectrons on the Nano-Femto Scale (Paperback, 1st ed. 2020)
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Imaging Light with Photoelectrons on the Nano-Femto Scale (Paperback, 1st ed. 2020)
Series: Springer Theses
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This thesis presents significant advances in the imaging and theory
of the ultrafast dynamics of surface plasmon polariton fields. The
author details construction of a sub-10 femtosecond and sub-10
nanometer spatiotemporal resolution ultrafast photoemission
microscope which is subsequently used for the discovery of
topological meron and skyrmion-like plasmonic quasiparticles. In
particular, this enabled the creation of movies of the surface
plasmon polariton fields evolving on sub-optical wavelength scales
at around 0.1 femtosecond per image frame undergoing vortex phase
evolution. The key insight that the transverse spin of surface
plasmon polaritons undergoes a texturing into meron or
skyrmion-like topological quasiparticles (defined by the geometric
charge of the preparation) follows. In addition, this thesis
develops an analytical theory of these new topological
quasiparticles, opening new avenues of research, while the
ultrafast microscopy techniques established within will also be
broadly applicable to studies of nanoscale optical excitations in
electronic materials.
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