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Books > Science & Mathematics > Chemistry > Physical chemistry > Quantum & theoretical chemistry
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State-to-State Dynamical Research in the F+H2 Reaction System (Paperback, 2014 ed.)
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State-to-State Dynamical Research in the F+H2 Reaction System (Paperback, 2014 ed.)
Series: Springer Theses
Expected to ship within 10 - 15 working days
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This thesis addresses two important and also challenging issues in
the research of chemical reaction dynamics of F+H2 system. One is
to probe the reaction resonance and the other is to determine the
extent of the breakdown of the Born-Oppenheimer approximation (BOA)
experimentally. The author introduces a state-of-the-art crossed
molecular beam-scattering apparatus using a hydrogen atom Rydberg
"tagging" time-of-flight method, and presents thorough
state-to-state experimental studies to address the above issues.
The author also describes the observation of the Feshbach resonance
in the F+H2 reaction, a precise measurement of the differential
cross section in the F+HD reaction, and validation of a new
accurate potential energy surface with spectroscopic accuracy.
Moreover, the author determines the reactivity ratio between the
ground state F(2P3/2) and the excited state F*(2P1/2) in the F+D2
reaction, and exploits the breakdown of BOA in the low collision
energy.
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