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Photoassociation of Ultracold CsYb Molecules and Determination of Interspecies Scattering Lengths (Hardcover, 1st ed. 2019)
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Photoassociation of Ultracold CsYb Molecules and Determination of Interspecies Scattering Lengths (Hardcover, 1st ed. 2019)
Series: Springer Theses
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This thesis lays the groundwork for producing a new class of
ultracold molecule by associating an alkali-metal atom and a
closed-shell alkaline-earth-like atom, specifically Cs and Yb. Such
molecules exhibit both a magnetic dipole moment and an electric
dipole moment in their ground state. This extra degree of freedom
opens up new avenues of research including the study of exotic
states of matter, the shielding of molecular collisions and the
simulation of lattice spin models. In detail, the thesis reports
the first and only ultracold mixture of Cs and Yb in the world,
giving details of the methods used to cool such contrasting atomic
species together. Using sensitive two-colour photoassociation
measurements to measure the binding energies of the near-threshold
CsYb molecular levels in the electronic ground state has allowed
the previously unknown scattering lengths to be accurately
determined for all the Cs-Yb isotopic combinations. As part of this
work, the one-photon photoassociation of ultracold Cs*Yb is also
studied, yielding useful information on the excited-state
potential. Knowledge of the scattering lengths enables a strategy
to be devised to cool both species to quantum degeneracy and,
crucially, determines the positions of interspecies Feshbach
resonances required for efficient association of ground-state CsYb
molecules. With these results, the prospect of bringing a new
molecule into the ultracold regime has become considerably closer.
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