Jonelle Harvey's book outlines two related experimental techniques,
threshold photoelectron spectroscopy and threshold photoelectron
photoion coincidence techniques, which are utilised to investigate
small halogenated molecules. All the experiments were conducted at
the vacuum ultraviolet beamline of the Swiss Light Source, a
synchrotron photon source, which has the advantage over popular
laser photon-sources of extreme ease of tunability. Three studies
are presented which combine experimental and computational ab
initio approaches: studying the fast dissociations of halogenated
methanes in order to construct a self-consistent thermochemical
network; investigating the fragmentations of fluoroethenes from
timebombs, which break apart very slowly but explosively, to fast
dissociators; and uncovering how vital conical interactions
underpin both the results of photoelectron spectra and dissociation
patterns. The details included in this thesis are useful for
researchers working in the same field and those readers wishing to
obtain a solid introduction into the types of systems encountered
in threshold photoelectron photoion coincidence spectroscopy.
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