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Ordering Phenomena in Rare-Earth Nickelate Heterostructures (Paperback, Softcover reprint of the original 1st ed. 2017)
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Ordering Phenomena in Rare-Earth Nickelate Heterostructures (Paperback, Softcover reprint of the original 1st ed. 2017)
Series: Springer Theses
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This thesis presents an experimental study of ordering phenomena in
rare-earth nickelate-based heterostructures by means of inelastic
Raman light scattering and elastic resonant x-ray scattering (RXS).
Further, it demonstrates that the amplitude ratio of magnetic
moments at neighboring nickel sites can be accurately determined by
RXS in combination with a correlated double cluster model, and
controlled experimentally through structural pinning of the oxygen
positions in the crystal lattice. The two key outcomes of the
thesis are: (a) demonstrating full control over the charge/bond and
spin order parameters in specifically designed praseodymium
nickelate heterostructures and observation of a novel spin density
wave phase in absence of the charge/bond order parameter, which
confirms theoretical predictions of a spin density wave phase
driven by spatial confinement of the conduction electrons; and (b)
assessing the thickness-induced crossover between collinear and
non-collinear spin structures in neodymium nickelate slabs, which
is correctly predicted by drawing on density functional theory.
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