This thesis reports results of precision mass spectrometry of
exotic nuclides as a means of elucidating their structure. The work
was performed with the ISOLTRAP spectrometer at CERN's ISOLDE
facility. The author furthermore offers an overview of existing
techniques used in Penning-trap mass spectrometry and also reports
on recent promising developments regarding ISOLTRAP. This
eloquently written treatment covers both theory and experiment, and
includes a general phenomenological introduction to the
nuclear-structure intuition contained in the trends of nuclear
binding energies.
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