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Studies of Photoinduced Molecular Dynamics Using a Fast Imaging Sensor (Hardcover, 1st ed. 2016)
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Studies of Photoinduced Molecular Dynamics Using a Fast Imaging Sensor (Hardcover, 1st ed. 2016)
Series: Springer Theses
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The work presented in this thesis involves a number of
sophisticated experiments highlighting novel applications of the
Pixel Imaging Mass Spectrometry (PImMS) camera in the field of
photoinduced molecular dynamics. This approach represents the union
of a new enabling technology (a multiple memory register,
CMOS-based pixel detector) with several modern chemical physics
approaches and represents a significant leap forward in
capabilities. Applications demonstrated include three-dimensional
imaging of photofragment Newton spheres, simultaneous electron-ion
detection using a single sensor, and ion-ion velocity correlation
measurements that open the door to novel covariance imaging
experiments. When combined with Coulomb explosion imaging, such an
approach is demonstrated to allow the measurement of molecular
structure and motion on a femtosecond timescale. This is
illustrated through the controlled photoexcitation of torsional
motion in biphenyl molecules and the subsequent real-time
measurement of the torsional angle.
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