The present work focuses on the development of intensified
small-scale extraction units for spent nuclear fuel reprocessing
using advanced process engineering with combined experimental and
modelling methodologies. It discusses a number of novel elements,
such as the intensification of spent fuel reprocessing and the use
of ionic liquids as green alternatives to organic solvents. The use
of ionic liquids in two-phase liquid-liquid separation is new to
the Multiphase Flow community, and has proved to be challenging,
especially in small channels, because of the surface and
interfacial properties involved, which are very different to those
of common organic solvents. Numerical studies have been also
performed to couple the hydrodynamics at small scale with the mass
transfer. The numerical results, taken together with scale-up
studies, are used to evaluate the applicability of the small-scale
units in reprocessing large volumes of nuclear waste.
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