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High Precision Optical Spectroscopy and Quantum State Selected Photodissociation of Ultracold 88Sr2 Molecules in an Optical Lattice (Hardcover, 1st ed. 2018)
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High Precision Optical Spectroscopy and Quantum State Selected Photodissociation of Ultracold 88Sr2 Molecules in an Optical Lattice (Hardcover, 1st ed. 2018)
Series: Springer Theses
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This thesis unites the fields of optical atomic clocks and
ultracold molecular science, laying the foundation for optical
molecular measurements of unprecedented precision. Building upon
optical manipulation techniques developed by the atomic clock
community, this work delves into attaining surgical control of
molecular quantum states. The thesis develops two experimental
observables that one can measure with optical-lattice-trapped
ultracold molecules: extremely narrow optical spectra, and angular
distributions of photofragments that are ejected when the diatomic
molecules are dissociated by laser light pulses. The former allows
molecular spectroscopy approaching the level of atomic clocks,
leading into molecular metrology and tests of fundamental physics.
The latter opens the field of ultracold chemistry through
observation of quantum effects such as matter-wave interference of
photofragments and tunneling through reaction barriers. The thesis
also describes a discovery of a new method of thermometry that can
be used near absolute zero temperatures for particles lacking
cycling transitions, solving a long-standing experimental problem
in atomic and molecular physics.
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