XUV Pump-Probe Experiments on Diatomic Molecules - Tracing the Dynamics of Electron Rearrangement and Interatomic Coulombic Decay (Hardcover, 2015 ed.)

This book explores the relaxation dynamics of inner-valence-ionized diatomic molecules on the basis of extreme-ultraviolet pump-probe experiments performed at the free-electron laser (FEL) in Hamburg. Firstly, the electron rearrangement dynamics in dissociating multiply charged iodine molecules is studied in an experiment that made it possible to access charge transfer in a thus far unexplored quasimolecular regime relevant for plasma and chemistry applications of the FEL. Secondly the lifetime of an efficient non-radiative relaxation process that occurs in weakly bound systems is measured directly for the first time in a neon dimer (Ne2). Interatomic Coulombic decay (ICD) has been identified as the dominant decay mechanism in inner-valence-ionized or excited van-der-Waals and hydrogen bonded systems, the latter being ubiquitous in all biomolecules. The role of ICD in DNA damage thus demands further investigation, e.g. with regard to applications like radiation therapy.

General

Imprint:	Springer International Publishing AG
Country of origin:	Switzerland
Series:	Springer Theses
Release date:	2015
First published:	2015
Authors:	Kirsten Schnorr
Dimensions:	235 x 155 x 13mm (L x W x T)
Format:	Hardcover
Pages:	191
Edition:	2015 ed.
ISBN-13:	978-3-319-12138-3
Categories:	Books > Science & Mathematics > Physics > Particle & high-energy physics Books > Science & Mathematics > Chemistry > Physical chemistry > Quantum & theoretical chemistry Books > Science & Mathematics > Chemistry > Analytical chemistry > Qualitative analytical chemistry > Chemical spectroscopy, spectrochemistry > General
LSN:	3-319-12138-3
Barcode:	9783319121383

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