In this thesis, the ionization of atoms and small molecules in strong laser fields is experimentally studied using a reaction microscope. The population of autoionizing doubly excited states in the laser fields is proven and a possible connection to the well-known dielectronic recombination processes is discussed. The fundamental process of tunnel ionization in strong laser fields is subject of investigation in a pump-probe experiment with ultrashort laser pulses. A coherent superposition of electronic states in singly charged argon ions is created within the first, and subsequently tunnel-ionized with the second pulse. This gives access to state-selective information about the tunneling process and allows to test common models. Moreover, the ionization of krypton and argon at different wavelengths is studied, from the multiphoton to the tunneling regime. The wavelength-dependent investigations are furthermore extended to molecular hydrogen. In addition to ionization, this system might undergo different dissociative processes. Channel-selective electron momentum distributions are presented and compared to each other.

This book covers the entire spectrum of the science and technology of nuclear reactor systems, from underlying physics, to next generation system applications and beyond. Beginning with neutron physics background and modeling of transport and diffusion, this self-contained learning tool progresses step-by-step to discussions of reactor kinetics, dynamics, and stability that will be invaluable to anyone with a college-level mathematics background wishing to develop an understanding of nuclear power. From fuels and reactions to full systems and plants, the author provides a clear picture of how nuclear energy works, how it can be optimized for safety and efficiency, and why it is important to the future.

This thesis represents a decisive breakthrough in our understanding of the physics of universal quantum-mechanical three-body systems. The Efimov scenario is a prime example of how fundamental few-body physics features universally across seemingly disparate fields of modern quantum physics. Initially postulated for nuclear physics more than 40 years ago, the Efimov effect has now become a new research paradigm not only in ultracold atomic gases but also in molecular, biological and condensed matter systems. Despite a lot of effort since its first observations, the scaling behavior, which is a hallmark property and often referred to as the "holy grail" of Efimov physics, remained hidden until recently. In this work, the author demonstrates this behavior for the first time for a heteronuclear mixture of ultracold Li and Cs atoms, and pioneers the experimental understanding of microscopic, non-universal properties in such systems. Based on the application of Born-Oppenheimer approximation, well known from molecular physics textbooks, an exceptionally clear and intuitive picture of heteronuclear Efimov physics is revealed.

This book will cover the cutting-edge developments in molecular and cellular mechanobiology to date. Readers will have a clear understanding of mechanobiology at the molecular and cellular levels, encompassing the mechanosensors, transducers, and transcription. An integrative approach across different scales from molecular sensing to mechanotransduction and gene modulation for physiological regulation of cellular functions will be explored, as well as applications to pathophysiological states in disease. A comprehensive understanding of the roles of physicochemical microenvironment and intracellular responses in determining cellular function in health and disease will also be discussed.

This book investigates elementary processes in the Earth's atmosphere involving photons, electrons, ions, radicals, and aerosols. It is based on global atmospheric models such as the standard atmospheric model with averaged atmospheric parameters across the globe and over time, the Earth's energetic balance, and the global electric circuit that allows to analyze fundamental atmospheric properties to be analyzed. Rate constants of elementary processes in the Earth's atmosphere, together with measured atmospheric parameters and existing concepts of atmospheric phenomena, are used in the analysis of global and local atmospheric processes. Atmospheric photoprocesses result from the interaction of solar radiation with the atmosphere and processes involving ions, oxygen atoms, excited atomic particles and ozone molecules. Atmospheric electricity as a secondary phenomenon to atmospheric water circulation results in a chain of processes that begins with collisions of water aerosols in different aggregate states. Cosmic rays are of importance for atmospheric electricity, as they create positive and negative ions in the air. Air breakdown in an electric field of clouds in the form of lightning may develop under the influence of cosmic ray-created seed electrons, which are necessary for electron multiplication in ionization wave-streamers. The upper atmosphere (ionosphere) is formed under solar radiation in a vacuum ultraviolet spectrum, and absorption of this radiation leads to air photoionization. The greenhouse effect is determined by atmospheric water, whereas transitions between a water vapor and aerosols may lead to a change in atmospheric optical depth. Carbon dioxide contributes in small portions to the atmospheric greenhouse effect. Cosmic rays are of importance for atmospheric discharge, the origin of lightning and cloud formation in the first stage of aerosol growth. This book provides a qualitative description of atmospheric properties and phenomena based on elementary processes and simple models.

This book displays the physics and design of high-power molecular lasers. The lasers described are self-controlled volume-discharge lasers. The book explains self-sustained discharge lasers, self-initiated discharge lasers and technical approaches to laser design. Important topics discussed are laser efficiency, laser beam quality and electric field homogeneity. The book contains many new innovative applications.

This book is devoted to theoretical methods used in the extreme circumstances of very strong electromagnetic fields. The development of high power lasers, ultrafast processes, manipulation of electromagnetic fields and the use of very fast charged particles interacting with other charges requires an adequate theoretical description. Because of the very strong electromagnetic field, traditional theoretical approaches, which have primarily a perturbative character, have to be replaced by descriptions going beyond them. In the book an extension of the semi-classical radiation theory and classical dynamics for particles is performed to analyze single charged atoms and dipoles submitted to electromagnetic pulses. Special attention is given to the important problem of field reaction and controlling dynamics of charges by an electromagnetic field.

This book features the latest advances and future trends in water science and technology. It also discusses the scientific popularization and quantitative resolution of a variety of mysterious properties of water and ice from the perspective of hydrogen-bond cooperativity in response to stimuli such as chemical contamination, electrification, magnetification, mechanical compression, molecular undercoordination, and thermal excitation. Anomalies include the floating of ice, the Hofmeister effect in solutions, regelation of ice, slipperiness of ice, water's tough skin, the Mpemba paradox, and the floating bridge. It also addresses the superfluidity of microchannels, hydrogen bond potentials, nanodroplet and bubble thermodynamics, quasisolidity and supersolidity, controlling superhydrophobicity-superhydrophilicity transition, and high-pressure ice formation. The target audience for this book includes students, senior scholars, engineers and practitioners in the area of physical chemistry, biology, as well as aqueous and colloid solutions.

This volume collects research findings presented at the 9th Edition of the Electronic Structure: Principles and Applications (ESPA-2014) International Conference, held in Badajoz, Spain, on July 2-4, 2014. The contributions cover research work on theory, methods and foundations, materials science, structure and chemical reactivity as well as environmental effects and modelling. Originally published in the journal Theoretical Chemistry Accounts, these outstanding papers are now available in a hardcover print format, as well as a special electronic edition. This volume provides valuable content for all researchers in theoretical chemistry, and will especially benefit those research groups and libraries with limited access to the journal.

This self-contained text introduces readers to the field of high-energy atomic physics - a new regime of photon-atom interactions in which the photon energies significantly exceed the atomic or molecular binding energies, and which opened up with the recent advent of new synchrotron sources. From a theoretical point of view, a small-parameter characteristic of the bound system emerged, making it possible to perform analytic perturbative calculations that can in turn serve as benchmarks for more powerful numerical computations. The first part of the book introduces readers to the foundations of this new regime and its theoretical treatment. In particular, the validity of the small-parameter perturbation expansion and of the lowest-order approximation is critically reviewed. The following chapters then apply these insights to various atomic processes, such as photoionization as a many-body problem, dominant mechanisms for the production of ions at higher energies, Compton scattering and ionization accompanied by creation of e-e+ pairs, and the photoionization of endohedral atoms (e.g. fullerene). Last but not least, the computationally challenging transitions in the electron shell during certain types of nuclear decays are investigated in detail.

This book is a complete treatment of work done to resolve the problems of position-, current-, and shape-control of plasma in tokamak-type (toroidal) devices being studied as a potential means of commercial energy production by nuclear fusion. Modelling and control are both detailed, allowing non-expert readers to understand the control problem. Starting from the magneto-hydro-dynamic equations, all the steps needed for the derivation of plasma state-space models are enumerated with frequent recall of the basic concepts of electromagnetics. The control problem is then described, beginning with the control of current and position-vertical and radial-control and progressing to the more challenging shape control. The solutions proposed vary from simple PIDs to more sophisticated MIMO controllers. The second edition of Magnetic Control of Tokamak Plasmas contains numerous updates and a substantial amount of completely new material covering areas such as: * modelling and control of resistive wall modes-the most important non-axisimmetric mode; * the isoflux approach for shape control; * a general approach for the control of limiter plasmas; * the use of inner vessel coils for vertical stabilization; and * significantly enhanced treatment of plasma-shape control at JET, including experimental results and introducing a method implemented for operation in the presence of current saturations. Whenever possible, coverage of the various topics is rounded out with experimental results obtained on currently existing tokamaks. The book also includes a presentation of the typical actuators and sensors used for control purposes in tokamaks. Some mathematical details are given in the appendices for the interested reader. The ideas formulated in this monograph will be of great practical help to control engineers, academic researchers and graduate students working directly with problems related to the control of nuclear fusion. They will also stimulate control researchers interested more generally in the advanced applications of the discipline. Advances in Industrial Control aims to report and encourage the transfer of technology in control engineering. The rapid development of control technology has an impact on all areas of the control discipline. The series offers an opportunity for researchers to present an extended exposition of new work in all aspects of industrial control.

This expanded and updated well-established textbook contains an advanced presentationof quantum mechanics adapted to the requirements of modern atomic physics. Itincludes topics of current interest such as semiclassical theory, chaos, atom optics andBose-Einstein condensation in atomic gases. In order to facilitate the consolidationof the material covered, various problems are included, together with completesolutions. The emphasis on theory enables the reader to appreciate the fundamentalassumptions underlying standard theoretical constructs and to embark on independentresearch projects. The fourth edition of Theoretical Atomic Physics contains anupdated treatment of the sections involving scattering theory and near-thresholdphenomena manifest in the behaviour of cold atoms (and molecules). Special attentionis given to the quantization of weakly bound states just below the continuum thresholdand to low-energy scattering and quantum reflection just above. Particular emphasisis laid on the fundamental differences between long-ranged Coulombic potentialsand shorter-ranged potentials falling off faster than 1/r2 at large distances r. The newsections on tunable near-threshold Feshbach resonances and on scattering in two spatialdimensions also address problems relevant for current and future research in the fieldof cold (and ultra-cold) atoms. Graduate students and researchers will find this book avaluable resource and comprehensive reference alike.

At the heart of this thesis is the young field of free electron laser science, whose experimental and theoretical basics are described here in a comprehensible manner. Extremely bright and ultra short pulses from short wavelength free-electron lasers (FELs) have recently opened the path to new fields of research. The x-ray flashes transform all matter into highly excited plasma states within femtoseconds, while their high spatial and temporal resolution allows the study of fast processes in very small structures. Even imaging of single molecules may be within reach if ultrafast radiation damage can be understood and brought under control. Atomic clusters have proven to be ideal model systems for light-matter interaction studies in all wavelength regimes, being size scalable, easy-to-produce gas phase targets with a simple structure. With FELs, "single cluster imaging and simultaneous ion spectroscopy" makes possible experiments under extremely well defined initial conditions, because the size of the cluster and the FEL intensity can be extracted from the scattering images. For the first time large xenon clusters up to micron radius were generated. Their single cluster scattering images were analyzed for cluster morphology and traces of the ultrafast plasma built-up during the femtosecond FEL pulse. The simultaneously measured single cluster ion spectra yield unprecedented insight into the ion dynamics following the interaction. The results will feed both future experimental effort and theoretical modeling.

This is the fifth volume in a series of Lecture Notes based on the highly successful Euro Summer School on Exotic Beams. The aim of these notes is to provide a thorough introduction to radioactive ion-beam physics at the level of graduate students and young postdocs starting out in the field. Each volume covers a range of topics from nuclear theory to experiment and applications. Vol I has been published as LNP 651, Vol II as LNP 700, Vol. III as LNP 764 and Vol. IV as LNP 879.

In this thesis Johanna Bruckner reports the discovery of the lyotropic counterpart of the thermotropic SmC* phase, which has become famous as the only spontaneously polarized, ferroelectric fluid in nature. By means of polarizing optical microscopy, X-ray diffraction and electro-optic experiments she firmly establishes aspects of the structure of the novel lyotropic liquid crystalline phase and elucidates its fascinating properties, among them a pronounced polar electro-optic effect, analogous to the ferroelectric switching of its thermotropic counterpart. The helical ground state of the mesophase raises the fundamental question of how chiral interactions are "communicated" across layers of more or less disordered and achiral solvent molecules which are located between adjacent bi-layers of the chiral amphiphile molecules. This thesis bridges an important gap between thermotropic and lyotropic liquid crystals and pioneers a new field of liquid crystal research.

The central subject of this thesis is the theoretical description of ultrafast dynamical processes in molecular systems of chemical interest and their control by laser pulses. This work encompasses different cutting-edge methods in quantum chemistry, quantum dynamics and for the rigorous description of the interaction of light and matter at the molecular level. It provides a general quantum mechanical framework for the description of chemical processes guided by laser pulses, in particular near conical intersections, i.e. geometries where the nuclear and electronic motions couple and the molecule undergoes non-adiabatic (or non-Born-Oppenheimer) dynamics. In close collaboration with experimentalists, the author succeeds in making a decisive step to link and to apply quantum physics to chemistry by transferring state of the art techniques and concepts developed in physics to chemistry, such as "light dressed atoms and molecules" and "adiabatic Floquet theory". He applies these techniques in three prototypic model systems (aniline, pyrazine and NHD2) using high-level electronic structure calculations. Readers will enjoy the comprehensive and accessible introduction to the topic and methodology, as well as the clear structure of the thesis.

The advent of laser-based sources of ultrafast infrared pulses has extended the study of very fast molecular dynamics to the observation of processes manifested through their effects on the vibrations of molecules. In addition, non-linear infrared spectroscopic techniques make it possible to examine intra- and intermolecular interactions and how such interactions evolve on very fast time scales, but also in some instances on very slow time scales. Ultrafast Infrared Vibrational Spectroscopy is an advanced overview of the field of ultrafast infrared vibrational spectroscopy based on the scientific research of the leading figures in the field. The book discusses experimental and theoretical topics reflecting the latest accomplishments and understanding of ultrafast infrared vibrational spectroscopy. Each chapter provides background, details of methods, and explication of a topic of current research interest. Experimental and theoretical studies cover topics as diverse as the dynamics of water and the dynamics and structure of biological molecules. Methods covered include vibrational echo chemical exchange spectroscopy, IR-Raman spectroscopy, time resolved sum frequency generation, and 2D IR spectroscopy. Edited by a recognized leader in the field and with contributions from top researchers, including experimentalists and theoreticians, this book presents the latest research methods and results. It will serve as an excellent resource for those new to the field, experts in the field, and individuals who want to gain an understanding of particular methods and research topics.

Why didn't the matter in our Universe annihilate with antimatter immediately after its creation? The study of CP violation may help to answer this fundamental question. This book presents theoretical tools necessary to understand this phenomenon. Reflecting the explosion of new results over the last decade, this second edition has been substantially expanded. It introduces charge conjugation, parity and time reversal, before describing the Kobayashi-Maskawa (KM) theory for CP violation and our understanding of CP violation in kaon decays. It reveals how the discovery of B mesons has provided a new laboratory to study CP violation with KM theory predicting large asymmetries, and discusses how these predictions have been confirmed since the first edition of this book. Later chapters describe the search for a new theory of nature's fundamental dynamics. This book is suitable for researchers in high energy, atomic and nuclear physics, and the history and philosophy of science.

This concise book provides the necessary background to allow interested readers to launch original research projects on the subject matter. Currently, this material is not available from one single source, and is either spread out over numerous journal publications, or covered in long and technical monographs. At the core of this book lies the sum rule approach to obtain analytic results in Quantum Chromodynamics (QCD), the current theory of strong interactions among quarks and gluons. This method fully complements Lattice QCD, the corresponding computational approach based on discretizing QCD on a space-time lattice. Applications include standard determinations of hadronic particle properties with extensions to finite temperature and density, and possibly involving the presence of extreme magnetic fields. The latter cases include stellar objects (e.g. neutron stars and magnetars) as well as high-energy proton-proton and heavy-ion collisions. Further topics concern the determination of the fundamental parameters of QCD, e.g. quark masses and the quark-gluon couplings, the hadronic contribution to the anomalous magnetic moment of the muon, and electromagnetic coupling at the the W-boson mass scale.

The book introduces the fundamentals of optical measurement mechanics, and discusses different types of interferometry, including (Digital) Holographic Interferometry, (Digital) Speckle Interferometry, Moire Interferometry, Digital Image Correlation and Particle Image Velocimetry. It is an essential reference for graduate students, scientists and practitioners from both universities and research laboratories.

This book provides the first complete and up-to-date summary of the state of the art in HAXPES and motivates readers to harness its powerful capabilities in their own research. The chapters are written by experts. They include historical work, modern instrumentation, theory and applications. This book spans from physics to chemistry and materials science and engineering. In consideration of the rapid development of the technique, several chapters include highlights illustrating future opportunities as well.

This book deals with the reflection of electromagnetic and particle waves by interfaces. The interfaces can be sharp or diffuse. The topics of the book contain absorption, inverse problems, anisotropy, pulses and finite beams, rough surfaces, matrix methods, numerical methods, reflection of particle waves and neutron reflection. Exact general results are presented, followed by long wave reflection, variational theory, reflection amplitude equations of the Riccati type, and reflection of short waves. The Second Edition of the Theory of Reflection is an updated and much enlarged revision of the 1987 monograph. There are new chapters on periodically stratified media, ellipsometry, chiral media, neutron reflection and reflection of acoustic waves. The chapter on anisotropy is much extended, with a complete treatment of the reflection and transmission properties of arbitrarily oriented uniaxial crystals. The book gives a systematic and unified treatment reflection and transmission of electromagnetic and particle waves at interfaces. It is intended for physicists, chemists, applied mathematicians and engineers, and is written in a simple direct style, with all necessary mathematics explained in the text.

This is the third edition of a well-known classic on ultrafast nonlinear and linear processes responsible for supercontinuum generation. Part I of the book reviews the progress achieved in experimental and theoretical understanding of the field, and goes over the applications developed since the discovery of the supercontinuum effect. The second part of the book covers recent research activity on supercontinuum phenomena and advances achieved since the publication of the previous edition. The new chapters specifically focus on: normal dispersion photonic band gap fibers; coherence in the supercontinuum; supercontinuum in the UV, NIR, and IR; and supercontinuum in XUV and X-rays for attosecond pulses. The Supercontinuum Laser Source is a definitive work by one of the discoverers of the white light effect. It is indispensable reading for any researcher or student working in the field of ultrafast laser physics.

Zeitschrift fur Kristallographie. Supplement Volume 38 presents the complete Abstracts of all contributions to the 26th Annual Conference of the German Crystallographic Society in Essen (Germany) 2018: - Plenary Talks - Microsymposia - Poster Session Supplement Series of Zeitschrift fur Kristallographie publishes Abstracts of international conferences on the interdisciplinary field of crystallography.

This in-depth textbook with a focus on atom-light interactions prepares students for research in a fast-growing and dynamic field. Intended to accompany the laser-induced revolution in atomic physics, it is a comprehensive text for the emerging era in atomic, molecular and optical science. Utilising an intuitive and physical approach, the text describes two-level atom transitions, including appendices on Ramsey spectroscopy, adiabatic rapid passage and entanglement. With a unique focus on optical interactions, the authors present multi-level atomic transitions with dipole selection rules, and M1/E2 and multiphoton transitions. Conventional structure topics are discussed in some detail, beginning with the hydrogen atom and these are interspersed with material rarely found in textbooks such as intuitive descriptions of quantum defects. The final chapters examine modern applications and include many references to current research literature. The numerous exercises and multiple appendices throughout enable advanced undergraduate and graduate students to balance theory with experiment.