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Books > Science & Mathematics > Physics > Atomic & molecular physics
The main goal of this book is to elucidate what kind of experiment must be performed in order to determine the full set of independent parameters which can be extracted and calculated from theory, where electrons, photons, atoms, ions, molecules, or molecular ions may serve as the interacting constituents of matter. The feasibility of such perfect' and-or `complete' experiments, providing the complete quantum mechanical knowledge of the process, is associated with the enormous potential of modern research techniques, both, in experiment and theory. It is even difficult to overestimate the role of theory in setting of the complete experiment, starting with the fact that an experiment can be complete only within a certain theoretical framework, and ending with the direct prescription of what, and in what conditions should be measured to make the experiment `complete'. The language of the related theory is the language of quantum mechanical amplitudes and their relative phases. This book captures the spirit of research in the direction of the complete experiment in atomic and molecular physics, considering some of the basic quantum processes: scattering, Auger decay and photo-ionization. It includes a description of the experimental methods used to realize, step by step, the complete experiment up to the level of the amplitudes and phases. The corresponding arsenal includes, beyond determining the total cross section, the observation of angle and spin resolved quantities, photon polarization and correlation parameters, measurements applying coincidence techniques, preparing initially polarized targets, and even more sophisticated methods. The `complete' experiment is, until today, hardly to perform. Therefore, much attention is paid to the results of state-of-the-art experiments providing detailed information on the process, and their comparison to the related theoretical approaches, just to mention relativistic multi-configurational Dirac-Fock, convergent close-coupling, Breit-Pauli R-matrix, or relativistic distorted wave approaches, as well as Green's operator methods. This book has been written in honor of Herbert Walther and his major contribution to the field but even to stimulate advanced Bachelor and Master students by demonstrating that obviously nowadays atomic and molecular scattering physics yields and gives a much exciting appreciation for further advancing the field.
The twelve chapters of this volume aim to provide a complete manual for using noble gases in terrestrial geochemistry, covering applications which range from high temperature processes deep in the Earth's interior to tracing climatic variations using noble gases trapped in ice cores, groundwaters and modern sediments. Other chapters cover noble gases in crustal (aqueous, CO2 and hydrocarbon) fluids and laboratory techniques for determining noble gas solubilities and diffusivities under geologically relevant conditions. Each chapter deals with the fundamentals of the analysis and interpretation of the data, detailing sampling and sampling strategies, techniques for analysis, sources of error and their estimation, including data treatment and data interpretation using recent case studies.
Based on a series of university lectures on nonrelativistic quantum mechanics, this textbook covers a wide range of topics, from the birth of quantum mechanics to the fine-structure levels of heavy atoms. The author sets out from the crisis in classical physics and explores the seminal ideas of Einstein, Bohr, and de Broglie and their vital importance for the development of quantum mechanics. There follows a bottom-up presentation of the postulates of quantum mechanics through real experiments (such as those of neutron interferometry), with consideration of their most important consequences, including applications in the field of atomic physics. A final chapter is devoted to the paradoxes of quantum mechanics, and particularly those aspects that are still open and hotly debated, to end up with a mention to Bell's theorem and Aspect's experiments. In presenting the principles of quantum mechanics in an inductive way, this book has already proved very popular with students in its Italian language version.It complements the exercises and solutions book "Problems in Quantum Mechanics", by E. d'Emilio, L.E. Picasso (Springer).
This corrected and updated second edition of "Scattering Theory" presents a concise and modern coverage of the subject. In the present treatment, special attention is given to the role played by the long-range behaviour of the projectile-target interaction, and a theory is developed, which is well suited to describe near-threshold bound and continuum states in realistic binary systems such as diatomic molecules or molecular ions. It is motivated by the fact that experimental advances have shifted and broadened the scope of applications where concepts from scattering theory are used, e.g. to the field of ultracold atoms and molecules, which has been experiencing enormous growth in recent years, largely triggered by the successful realization of Bose-Einstein condensates of dilute atomic gases in 1995. The book contains sections on special topics such as near-threshold quantization, quantum reflection, Feshbach resonances and the quantum description of scattering in two dimensions. The level of abstraction is kept as low as at all possible and deeper questions related to the mathematical foundations of scattering theory are passed by. It should be understandable for anyone with a basic knowledge of nonrelativistic quantum mechanics. The book is intended for advanced students and researchers, and it is hoped that it will be useful for theorists and experimentalists alike.
This book is a complete update of the classic 1981 FAST BREEDER REACTORS textbook authored by Alan E. Waltar and Albert B. Reynolds, which , along with the Russian translation, served as a major reference book for fast reactors systems. Major updates include transmutation physics (a key technology to substantially ameliorate issues associated with the storage of high-level nuclear waste ), advances in fuels and materials technology (including metal fuels and cladding materials capable of high-temperature and high burnup), and new approaches to reactor safety (including passive safety technology), New chapters on gas-cooled and lead-cooled fast spectrum reactors are also included. Key international experts contributing to the text include Chaim Braun, (Stanford University) Ronald Omberg, (Pacific Northwest National Laboratory, Massimo Salvatores (CEA, France), Baldev Raj, (Indira Gandhi Center for Atomic Research, India) , John Sackett (Argonne National Laboratory), Kevan Weaver, (TerraPower Corporation) ,James Seinicki(Argonne National Laboratory). Russell Stachowski (General Electric), Toshikazu Takeda (University of Fukui, Japan), and Yoshitaka Chikazawa (Japan Atomic Energy Agency).
The second edition of "The Chemistry of the Superheavy Elements" provides a complete coverage of the chemistry of a series of elements beginning with atomic number 104 - the transactinides or superheavy elements - including their nuclear properties and production in nuclear reactions at heavy-ion accelerators. The contributors to this work include many renowned scientists who, during the last decades, have made vast contributions towards understanding the physics and chemistry of these elusive elements, both experimentally and theoretically. The main emphasis here is on demonstrating the fascinating studies involved in probing the architecture of the Periodic Table at its uppermost end, where relativistic effects drastically influence chemical properties. All known chemical properties of these elements are described together with the experimental techniques applied to study these short-lived man-made elements one atom-at-a-time. The status of theoretical chemistry and of empirical models is presented as well as aspects of nuclear physics. In addition, one chapter outlines the meanderings in this field from a historical perspective and the search for superheavy elements in Nature.
Novel coherent light sources such as x-ray free-electron lasers open exciting prospects for the interaction of light with nuclei. The thesis "Coherent Control of Nuclei and X-rays" covers this still-developing field and proposes, in a daring attempt to revolutionize nuclear physics, three innovative schemes for taming nuclei using coherent effects. The theoretical explorations, which address control of nuclear quantum states, a nuclear memory for single photons in future photonic circuits, and optimized concepts for a nuclear clock, make use of new approaches at the borderline between nuclear physics and quantum dynamics. The result is a well written work, impressive in its stimulating style and promising ideas.
This exhaustive survey is the result of a four year effort by many leading researchers in the field to produce both a readable introduction and a yardstick for the many upcoming experiments using heavy ion collisions to examine the properties of nuclear matter. The books falls naturally into five large parts, first examining the bulk properties of strongly interacting matter, including its equation of state and phase structure. Part II discusses elementary hadronic excitations of nuclear matter, Part III addresses the concepts and models regarding the space-time dynamics of nuclear collision experiments, Part IV collects the observables from past and current high-energy heavy-ion facilities in the context of the theoretical predictions specific to compressed baryonic matter. Part V finally gives a brief description of the experimental concepts. The book explicitly addresses everyone working or planning to enter the field of high-energy nuclear physics.
Optical Coherence Tomography represents the ultimate noninvasive ocular imaging technique although being in the field for over two-decades. This book encompasses both medical and technical developments and recent achievements. Here, the authors cover the field of application from the anterior to the posterior ocular segments (Part I) and present a comprehensive review on the development of OCT. Important developments towards clinical applications are covered in Part II, ranging from the adaptive optics to the integration on a slit-lamp, and passing through new structural and functional information extraction from OCT data. The book is intended to be informative, coherent and comprehensive for both the medical and technical communities and aims at easing the communication between the two fields and bridging the gap between the two scientific communities.
This book gives a detailed overview of the theory of electromagnetic wave scattering on single, homogeneous, but nonspherical particles. Beside the systematically developed Green’s function formalism of the first edition this second and enlarged edition contains additional material regarding group theoretical considerations for nonspherical particles with boundary symmetries, an iterative T-matrix scheme for approximate solutions, and two additional but basic applications. Moreover, to demonstrate the advantages of the group theoretical approach and the iterative solution technique, the restriction to axisymmetric scatterers of the first edition was abandoned.
Various experimental techniques have been advanced in recent years to measure non-equilibrium energy transformations on the microscopic scale of single molecules. In general, the systems studied in the corresponding experiments are exposed to strong thermal fluctuations and thus the relevant energetic variables such as work and heat become stochastic. This thesis addresses challenging theoretical problems in this active field of current research: 1) Exact analytical solutions of work and heat distributions for isothermal non-equilibrium processes in suitable models are obtained; 2) Corresponding solutions for cyclic processes involving two different heat reservoirs are found; 3) Optimization of periodic driving protocols for such cyclic processes with respect to maximal output power, efficiency and minimal power fluctuations is studied. The exact solutions for work and heat distributions provide a reference for theoretical investigations of more complicated models, giving insight into the structure of the tail of work distributions and serving as valuable test cases for simulations of the underlying stochastic processes.
In this thesis, the measurement of double-spin asymmetry for electron production from heavy flavor decays was performed in a Relativistic Heavy Ion Collider (RHIC) in the PHENIX experiment at Brookhaven National Laboratory to measure the polarized parton distribution function of gluon in the small Bjorken x region (x~0.01). Â For this experiment, for the first time a Hadron Blind Detector (HBD), which is a position-sensitive gas Cherenkov counter with Gas Electron Multiplier whose surface is evaporated by CsI, was employed. This HBD contributes to reducing the background from electron pairs produced by real and virtual photon conversion. Furthermore, the author develops a new analysis method for the background reduction, and the signal-to-background ratio is improved by a factor of roughly 2.0. Using the combination of the HBD and a new analysis method, the double-spin asymmetry of the electron production with transverse momentum ranging 0.5 < pT < 3.0 GeV/c is measured and confirmed to be zero-consistent within the limit of the statistical uncertainty of about 1%. This result identifies the constraint of the gluon polarization in the small Bjorken x region, a worldwide first.
This volume collects research findings presented at the 8th Edition of the Electronic Structure: Principles and Applications (ESPA-2012) International Conference, held in Barcelona, Spain on June 26-29, 2012. The contributions cover research work on methods and fundamentals of theoretical chemistry, chemical reactivity, bimolecular modeling, and materials science. Originally published in the journal Theoretical Chemistry Accounts, these outstanding papers are now available in a hardcover print format, as well as a special electronic edition. This volume provides valuable content for all researchers in theoretical chemistry, and will especially benefit those research groups and libraries with limited access to the journal.
It has been suggested that local parity violation (LPV) in Quantum Chromodynamics (QCD) would lead to charge separation of quarks by the Chiral Magnetic Effect (CME) in heavy ion collisions. Charge Multiplicity Asymmetry Correlation Study Searching for Local Parity Violation at RHIC for STAR Collaboration presents the detailed study of charge separation with respect to the event plane. Results on charge multiplicity asymmetry in Au+Au and d+Au collisions at 200 GeV by the STAR experiment are reported. It was found that the correlation results could not be explained by CME alone. Additionally, the charge separation signal as a function of the measured azimuthal angle range as well as the event-by-event anisotropy parameter are studied. These results indicate that the charge separation effect appears to be in-plane rather than out-of-plane. It is discovered that the charge separation effect is proportional to the event-by-event azimuthal anisotropy and consistent with zero in events with zero azimuthal anisotropy. These studies suggest that the charge separation effect, within the statistical error, may be a net effect of event anisotropy and correlated particle production. A potential upper limit on the CME is also presented through this data.
Our understanding of nature, and in particular of physics and the laws governing it, has changed radically since the days of the ancient Greek natural philosophers. This book explains how and why these changes occurred, through landmark experiments as well as theories that - for their time - were revolutionary. The presentation covers Mechanics, Optics, Electromagnetism, Thermodynamics, Relativity Theory, Atomic Physics and Quantum Physics. The book places emphasis on ideas and on a qualitative presentation, rather than on mathematics and equations. Thus, although primarily addressed to those who are studying or have studied science, it can also be read by non-specialists. The author concludes with a discussion of the evolution and organization of universities, from ancient times until today, and of the organization and dissemination of knowledge through scientific publications and conferences.
This dissertation focuses on the calculation of transport coefficients in the matter created in a relativistic heavy-ion collision after chemical freeze-out. This matter can be well approximated using a pion gas out of equilibrium. We describe the theoretical framework needed to obtain the shear and bulk viscosities, the thermal and electrical conductivities and the flavor diffusion coefficients of a meson gas at low temperatures. To describe the interactions of the degrees of freedom, we use effective field theories with chiral and heavy quark symmetries. We subsequently introduce the unitarization methods in order to obtain a scattering amplitude that satisfies the unitarity condition exactly, then go on to calculate the transport properties of the low-temperature phase of quantum chromodynamics - the hadronic medium - which can be used in hydrodynamic simulations of a relativistic heavy-ion collision and its subsequent evolution. We show that the shear viscosity over entropy density exhibits a minimum in a phase transition by studying this coefficient in atomic Argon (around the liquid-gas phase transition) and in the linear sigma model in the limit of a large number of scalar fields (which presents a chiral phase transition). Finally, we provide an experimental method for estimating the bulk viscosity in relativistic heavy-ion collisions by performing correlations of the fluctuating components of the stress-energy tensor.
This multi-author contributed volume includes methodological advances and original applications to actual chemical or biochemical phenomena which were not possible before the increased sophistication of modern computers. The chapters contain detailed reviews of the developments of various computational techniques, used to study complex molecular systems such as molecular liquids and solutions (particularly aqueous solutions), liquid-gas, solid-gas interphase and biomacromolecular systems. Quantum modeling of complex molecular systems is a useful resource for graduate students and fledgling researchers and is also an excellent companion for research professionals engaged in computational chemistry, material science, nanotechnology, physics, drug design, and molecular biochemistry.
This book presents the basics and advanced topics of research of gamma ray physics. It describes measuring of Fermi surfaces with gamma resonance spectroscopy and the theory of angular distributions of resonantly scattered gamma rays. The dependence of excited-nuclei average lifetime on the shape of the exciting-radiation spectrum and electron binding energies in the spectra of scattered gamma rays is described. Resonant excitation by gamma rays of nuclear isomeric states with long lifetime leads to the emission and absorption lines. In the book, a new gamma spectroscopic method, gravitational gamma spectrometry, is developed. It has a resolution hundred million times higher than the usual Moessbauer spectrometer. Another important topic of this book is resonant scattering of annihilation quanta by nuclei with excited states in connection with positron annihilation. The application of the methods described is to explain the phenomenon of Coulomb fragmentation of gamma-source molecules and resonant scattering of annihilation quanta to study the shape of Fermi surfaces of metals.
This textbook explains the experimental basics, effects and theory of nuclear physics. It supports learning and teaching with numerous worked examples, questions and problems with answers. Numerous tables and diagrams help to better understand the explanations. A better feeling to the subject of the book is given with sketches about the historical development of nuclear physics. The main topics of this book include the phenomena associated with passage of charged particles and radiation through matter which are related to nuclear resonance fluorescence and the Moessbauer effect., Gamov's theory of alpha decay, Fermi theory of beta decay, electron capture and gamma decay. The discussion of general properties of nuclei covers nuclear sizes and nuclear force, nuclear spin, magnetic dipole moment and electric quadrupole moment. Nuclear instability against various modes of decay and Yukawa theory are explained. Nuclear models such as Fermi Gas Model, Shell Model, Liquid Drop Model, Collective Model and Optical Model are outlined to explain various experimental facts related to nuclear structure. Heavy ion reactions, including nuclear fusion, are explained. Nuclear fission and fusion power production is treated elaborately.
The aim of this book is to present highly accurate and extensive theoretical Atomic data and to give a survey of selected calculational methods for atomic physics, used to obtain these data. The book presents the results of calculations of cross sections and probabilities of a broad variety of atomic processes with participation of photons and electrons, namely on photoabsorption, electron scattering and accompanying effects. Included are data for photoabsorption and electron scattering cross-sections and probabilities of vacancy decay formed for a large number of atoms and ions. Attention is also given to photoionization and vacancy decay in endohedrals and to positron-atom scattering. The book is richly illustrated. The methods used are one-electron Hartree-Fock and the technique of Feynman diagrams that permits to include many-electron correlations. This is done in the frames of the Random Phase approximation with exchange and the many-body perturbation theory. Newly obtained and previously collected atomic data are presented. The atomic data are useful for investigating the electronic structure and physical processes in solids and liquids, molecules and clusters, astronomical objects, solar and planet atmospheres and atomic nucleus. Deep understanding of chemical reactions and processes is reached by deep and accurate knowledge of atomic structure and processes with participation of atoms. This book is useful for theorists performing research in different domains of contemporary physics, chemistry and biology, technologists working on production of new materials and for experimentalists performing research in the field of photon and electron interaction with atoms, molecules, solid bodies and liquids.
Janne Marie Soetbeer determines the optimal dynamical decoupling (DD) scheme for efficient reduction of electron spin coherence loss in model systems for spin labelled biomolecules depending on their particular relaxation behavior. Extending the nth order DD scheme to double electron-electron resonance (DEER) experiments require the addition of multiple pump pulses for 1. Incomplete excitation of pump spin packets introduce signal artefacts which are minimized by pump pulse optimization including linear-chirp and asymmetric hyperbolic secant pulses. Prolonging the dipolar evolution time with decreased signal artefact allows to extent the measurable interspin distances in biomolecules which were otherwise not accessible due to spin echo relaxation.
"This book contains overviews on technologically important classes of glasses, their treatment to achieve desired properties, theoretical approaches for the description of structure-property relationships, and new concepts in the theoretical treatment of crystallization in glass-forming systems. It contains overviews about the state of the art and about specific features for the analysis and application of important classes of glass-forming systems, and describes new developments in theoretical interpretation by well-known glass scientists. Thus, the book offers comprehensive and abundant information that is difficult to come by or has not yet been made public." Edgar Dutra Zanotto (Center for Research, Technology and Education in Vitreous Materials, Brazil) Glass, written by a team of renowned researchers and experienced book authors in the field, presents general features of glasses and glass transitions. Different classes of glassforming systems, such as silicate glasses, metallic glasses, and polymers, are exemplified. In addition, the wide field of phase formation processes and their effect on glasses and their properties is studied both from a theoretical and experimental point of view.
The most complete introduction available to molecular dynamics and
the calculation of rate of reaction
This graduate textbook introduces the com-putational techniques to study ultra-fast quantum dynamics of matter exposed to strong laser fields. Coverage includes methods to propagate wavefunctions according to the time dependent Schroedinger, Klein-Gordon or Dirac equation, the calculation of typical observables, time-dependent density functional theory, multi configurational time-dependent Hartree-Fock, time-dependent configuration interaction singles, the strong-field approximation, and the microscopic particle-in-cell approach. Contents How to propagate a wavefunction? Calculation of typical strong-field observables Time-dependent relativistic wave equations: Numerics of the Dirac and the Klein-Gordon equation Time-dependent density functional theory The multiconfiguration time-dependent Hartree-Fock method Time-dependent configuration interaction singles Strong-field approximation and quantum orbits Microscopic particle-in-cell approach
This brief discusses the mechanism of functional expression of a protein or protein complex utilizing the ATP hydrolysis cycle or proton-motive force from a unique point of view focused on the roles of water. A variety of processes are considered such as the unidirectional movement of a linear-motor protein along a filament, insertion of an unfolded protein into a chaperonin and release of the folded protein from it, transport of diverse substrates across the membrane by a transporter, and directed rotation of the central subunit within a rotatory motor protein complex. These topics are discussed in a unified manner within the same theoretical framework. The author argues that water plays imperative roles in the functional expression of these molecular machines. A pivotal factor is the entropic force or potential originating from the translational displacement of water molecules coexisting with the molecular machines in the entire system. |
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