Systems of trapped ions and systems of ultracold Rydberg atoms are used at the forefront of quantum physics research and they make strong contenders as platforms for quantum technologies. Trapped Rydberg ions are a new hybrid technology envisaged to have both the exquisite control of trapped ion systems and the strong interactions of Rydberg atoms. In this work a single trapped Rydberg ion is experimentally investigated. A trapped strontium ion is excited to Rydberg states using two ultraviolet lasers. Effects of the strong trapping electric fields on the highly-sensitive Rydberg ion are studied. After mitigating unwanted trap effects, the ion is coherently excited to Rydberg states and a quantum gate is demonstrated. This thesis lays much of the experimental groundwork for research using this novel system.

This book introduces vibronic coupling density and vibronic coupling constant analyses as a way to understand molecular structure and chemical reactions. After quantum study, the behavior of electrons circulating around nuclei led to the principal concept that underlies all explanations in chemistry. Many textbooks have given plausible explanations to clarify molecular structure-for example, the bond elongation of ethylene under anionization and the nonplanar structure of ammonia. Frontier molecular orbital concepts were proposed to visualize the path of chemical reactions, and conventional explanations gave students a familiarity with molecular structures in terms of the electronic state. By contrast, this book offers a more rational and more convincing path to understanding. It starts from the ab initio molecular Hamiltonian and provides systematic, rational approaches to comprehend chemical phenomena. In this way, the book leads the reader to a grasp of the quantitative evaluation of the force applied under the molecular deformation process. As well, guidelines are offered for integrating the traditional "hand-waving" approach of chemistry with more rational and general VCD and VCC alternatives along with the outlook for newly functionalized chemical systems.

Fusion neutron sources have many important practical uses, such as irradiation testing of materials and components, facilitating the production of various isotopes such as tritium, driving subcritical cores, characterizing spent nuclear fuel, and manufacturing medical isotopes. All these applications can be potentially improved by achieving higher neutron yields and fluxes in compact fusion neutron sources (CFNSs). This publication is a compilation arising from an IAEA coordinated research project on this topic and presents the project's main results and findings with the aim of supporting stakeholders in the development of CFNSs in the transition from conceptual to engineering design.

Management systems play an important role in the success of a nuclear power programme. Recognizing that their development poses a number of questions, this publication aims to share experiences of regulatory bodies and owner operator organizations in developing management systems consistent with the main activities planned from inception of these organizations to construction of a nuclear power plant, whilst prioritizing safety.

This book describes advanced research on the structures and photochemical properties of polyatomic molecules and molecular clusters having various functionalities under cold gas-phase conditions. Target molecules are crown ethers, polypeptides, large size protonated clusters, metal clusters, and other complex polyatomic molecules of special interest. A variety of advanced frequency and time-domain laser spectroscopic methods are applied. The book begins with the principle of an experimental setup for cold gas-phase molecules and various laser spectroscopic methods, followed by chapters on investigation of specific molecular systems. Through a molecular-level approach and analysis by quantum chemical calculation, it is possible to learn how atomic and molecular-level interactions (van der Waals, hydrogen-bonding, and others) control the specific properties of molecules and clusters. Those properties include molecular recognition, induced fitting, chirality, proton and hydrogen transfer, isomerization, and catalytic reaction. The information will be applicable to the design of new types of functional molecules and nanoparticles in the broad area that includes applied chemistry, drug delivery systems, and catalysts.

This book focuses on the study of the interfacial water using molecular dynamics simulation and experimental sum frequency generation spectroscopy. It proposes a new definition of the free O-H groups at water-air interface and presents research on the structure and dynamics of these groups. Furthermore, it discusses the exponential decay nature of the orientation distribution of the free O-H groups of interfacial water and ascribes the origin of the down pointing free O-H groups to the presence of capillary waves on the surface. It also describes how, based on this new definition, a maximum surface H-bond density of around 200 K at ice surface was found, as the maximum results from two competing effects. Lastly, the book discusses the absorption of water molecules at the water-TiO2 interface. Providing insights into the combination of molecular dynamics simulation and experimental sum frequency generation spectroscopy, it is a valuable resource for researchers in the field.

This book provides a systematic and comprehensive introduction to the neutronics of advanced nuclear systems, covering all key aspects, from the fundamental theories and methodologies to a wide range of advanced nuclear system designs and experiments. It is the first-ever book focusing on the neutronics of advanced nuclear systems in the world. Compared with traditional nuclear systems, advanced nuclear systems are characterized by more complex geometry and nuclear physics, and pose new challenges in terms of neutronics. Based on the achievements and experiences of the author and his team over the past few decades, the book focuses on the neutronics characteristics of advanced nuclear systems and introduces novel neutron transport methodologies for complex systems, high-fidelity calculation software for nuclear design and safety evaluation, and high-intensity neutron source and technologies for neutronics experiments. At the same time, it describes the development of various neutronics designs for advanced nuclear systems, including neutronics design for ITER, CLEAR and FDS series reactors. The book not only summarizes the progress and achievements of the author's research work, but also highlights the latest advances and investigates the forefront of the field and the road ahead.

This book highlights the latest advances and outlines future trends in aqueous solvation studies from the perspective of hydrogen bond transition by charge injection, which reconciles the solvation dynamics, molecular nonbond interactions, and the extraordinary functionalities of various solutes on the solution bond network and properties. Focus is given on ionic and dipolar electrostatic polarization, O:H nonbond interaction, anti-HB and super-HB repulsion, and solute-solute interactions. Its target audience includes researchers, scientists, and engineers in chemistry, physics, surface and interface science, materials science and engineering.

The present research studies the fundamental physics occurring during the magnetic flux and magnetized plasma compression by plasma implosion. This subject is relevant to numerous studies in laboratory and space plasmas. Recently, it has attracted particular interest due to the advances in producing high-energy-density plasmas in fusion-oriented experiments, based on the approach of magnetized plasma compression. The studied configuration consists of a cylindrical gas-puff shell with pre-embedded axial magnetic field that pre-fills the anode-cathode gap. Subsequently, axial pulsed current is driven through the plasma generating an azimuthal magnetic field that compresses the plasma and the axial magnetic field embedded in it. A key parameter for the understanding of the physics occurring during the magnetized plasma compression is the evolution and distribution of the axial and azimuthal magnetic fields. Here, for the first time ever, both fields are measured simultaneously employing non-invasive spectroscopic methods that are based on the polarization properties of the Zeeman effect. These measurements reveal unexpected results of the current distribution and the nature of the equilibrium between the axial and azimuthal fields. These observations show that a large part of the current does not flow in the imploding plasma, rather it flows through a low-density plasma residing at large radii. The development of a force-free current configuration is suggested to explain this phenomenon. Previously unpredicted observations in higher-power imploding-magnetized-plasma experiments, including recent unexplained structures observed in the Magnetized Liner Inertial Fusion experiment, may be connected to the present discovery.

X ray, neutron and gamma radiography have been widely used by industry as non-destructive testing methods for quality control and to assess the safety and integrity of structures. Such techniques use intense, human-made radiation sources in the laboratory and at industrial sites. Muons are relatively massive elementary particles produced naturally by cosmic rays, and which may be used as a highly penetrating, non-destructive probe. Muon imaging is therefore an attractive alternative for certain applications. This publication describes some of the main muon imaging techniques, the detector types involved, and a wide variety of applications that have been identified from examination of modern and ancient built environments, volcanology, industry to nuclear security and safeguards. This publication is expected to be of use to all those individuals working in industry and academia with an interest in muon imaging.

Scattering theory provides a framework for understanding the scattering of waves and particles. This book presents a simple physical picture of diffractive nuclear scattering in terms of semi-classical trajectories, illustrated throughout with examples and case studies. Trajectories in a complex impact parameter plane are discussed, and it stresses the importance of the analytical properties of the phase shift function in this complex impact plane in the asymptotic limit. Several new rainbow phenomena are also discussed and illustrated. Written by Nobel Prize winner Roy J. Glauber, and Per Osland, an expert in the field of particle physics, the book illustrates the transition from quantum to classical scattering, and provides a valuable resource for researchers using scattering theory in nuclear, particle, atomic and molecular physics.

The interactions of DNA with force are central to manifold fields of inquiry, including the de novo design of DNA nanostructures, the use of DNA to probe the principles of biological self-assembly, and the operation of cellular nanomachines. This work presents a survey of three distinct ways coarse-grained simulations can help characterize these interactions. A non-equilibrium energy landscape reconstruction technique is validated for use with the oxDNA model and a practical framework to guide future applications is established. A novel method for calculating entropic forces in DNA molecules is outlined and contrasted with existing, flawed approaches. Finally, a joint experimental-simulation study of large DNA origami nanostructures under force sheds light on design principles and, through vivid illustrations, their unfolding process. This text provides an accessible and exciting launching point for any student interested in the computational study of DNA mechanics and force interactions.

This INSAG report defines in detail the independence needed in the regulatory decision making process and how to meet the potential challenges to that independence. Thus, the report identifies a number of measures that need to be implemented at different levels to promote and protect independence in the regulatory decision making process. The basic principles have to be embedded into the legal framework and followed up by systematic quality management of regulatory processes and activities.

This primer begins with a brief introduction to the main ideas underlying Effective Field Theory (EFT) and describes how nuclear forces are obtained from first principles by introducing a Euclidean space-time lattice for chiral EFT. It subsequently develops the related technical aspects by addressing the two-nucleon problem on the lattice and clarifying how it fixes the numerical values of the low-energy constants of chiral EFT. In turn, the spherical wall method is introduced and used to show how improved lattice actions render higher-order corrections perturbative. The book also presents Monte Carlo algorithms used in actual calculations. In the last part of the book, the Euclidean time projection method is introduced and used to compute the ground-state properties of nuclei up to the mid-mass region. In this context, the construction of appropriate trial wave functions for the Euclidean time projection is discussed, as well as methods for determining the energies of the low-lying excitations and their spatial structure. In addition, the so-called adiabatic Hamiltonian, which allows nuclear reactions to be precisely calculated, is introduced using the example of alpha-alpha scattering. In closing, the book demonstrates how Nuclear Lattice EFT can be extended to studies of unphysical values of the fundamental parameters, using the triple-alpha process as a concrete example with implications for the anthropic view of the Universe. Nuclear Lattice Effective Field Theory offers a concise, self-contained, and introductory text suitable for self-study use by graduate students and newcomers to the field of modern computational techniques for atomic nuclei and nuclear reactions.

This publication has been produced as part of the IAEA's Modelling and Data for Radiological Impact Assessments (MODARIA) programme. It summarizes the activities of Working Group 7, which was one of ten working groups within MODARIA, and focused on the harmonization and intercomparison of models for the accidental release of tritium to the atmosphere. It addresses the modelling of tritium into the atmosphere and the subsequent terrestrial processes that determine the dynamic transfer of tritium in the environment. The first half of the report contains a literature review regarding state-of-the-art modelling of tritium in the terrestrial environment. The second half summarizes the results of an intercomparison exercise undertaken using four models to inform the direction of future research.

The response of a nuclear installation's structure during an earthquake depends on the characteristics of the ground motion, the surrounding soil and the structure itself. Soil– structure interaction (SSI) analysis is used to evaluate the effects of seismic ground motion on an installation's structure, system and components, to ensure it is designed to withstand the effects of earthquakes, without loss of safety functions. This publication presents SSI phenomena and current practices in SSI modelling, simulation methodology and analysis methods for the design and assessment of nuclear installations. It complements IAEA Safety Standards Series No. SSG-67, Seismic Design for Nuclear Installations, and No. NS-G-2.13, Evaluation of Seismic Safety for Existing Nuclear Installations.

This book reviews various aspects of molecular spectroscopy and its application in materials science, chemistry, physics, medicine, the arts and the earth sciences. Written by an international group of recognized experts, it examines how complementary applications of diverse spectroscopic methods can be used to study the structure and properties of different materials. The chapters cover the whole spectrum of topics related to theoretical and computational methods, as well as the practical application of spectroscopic techniques to study the structure and dynamics of molecular systems, solid-state crystalline and amorphous materials, surfaces and interfaces, and biological systems. As such, the book offers an invaluable resource for all researchers and postgraduate students interested in the latest developments in the theory, experimentation, measurement and application of various advanced spectroscopic methods for the study of materials.

This book is based on Valery Zagrebaev's original papers and lecture materials on nuclear physics with heavy ions, which he prepared and extended through many years for the students of nuclear physics specialties. Th book outlines the main experimental facts on nuclear reactions involving heavy ions at low energies. It focuses on discussions of nuclear physics processes that are a subject of active, modern research and it gives illustrative explanations of these phenomena in the framework of up-to-date theoretical concepts. This textbook is intended for students in physics who have completed a standard course of quantum mechanics and have basic ideas of nuclear physics processes. It is designed as a kind of lifeboat that, at the end of the course, will allow students to navigate the modern scientific literature and to understand the goals and objectives of current, on-going research.

This publication provides guidance to States and their competent authorities on how to implement and maintain a physical protection regime for transport of nuclear material. It will also be useful to shippers or carriers in the design and implementation of their physical protection systems. The publication builds upon IAEA Nuclear Security Series No. 13, Nuclear Security Recommendations on Physical Protection of Nuclear Material and Nuclear Facilities (INFCIRC/225/Revision 5), and provides additional guidance on how to implement these recommendations in practice.

Part 1: A Dostoeyevskijan Hero.- An Archimedes from Sicily studies in Rome.- A Certain Interest in Pure Science.- Ten short papers.- Part 2: Power for the Italian School.- The 1937 Chance.- Landing in Naples.- Part 3: A Legacy from the Grand Inquisitor.- The Mystery of the Missing Papers.- Fortunes and Misfortunes of a Famous Director.- Part 4: Investigation of a Disappearance.- Before March 26.- In Search for a Missing Professor.- The Last Chapter.- Epilogue.

A number of IAEA Member States generate relatively small quantities of radioactive waste and/or disused sealed sources in research or in the application of nuclear techniques in medicine and industry. This publication presents a modular approach to the design of waste processing and storage facilities to address the needs of such Member States with a cost effective and flexible solution that allows easy adjustment to changing needs in terms of capacity and variety of waste streams. The key feature of the publication is the provision of practical guidance to enable the users to determine their waste processing and storage requirements, specify those requirements to allow the procurement of the appropriate processing and storage modules and install and eventually operate those modules.

Rising operating costs and increased competition have focused attention on the need to improve thermal performance in nuclear power plants (NPPs), to ensure efficient electricity generation. Efforts to improve thermal performance require a broad understanding of NPP design, operation, maintenance, ambient conditions, and thermal sciences. This publication provides various methodologies for tracking and trending NPP thermal performance. It describes the essential elements of a thermal performance programme, providing guidelines on the design of the balance of the plant systems for new build NPPs and improvements to an existing programme for operating NPPs.

Gamma-ray bursts (GRBs) are the most luminous explosions in the universe, which within seconds release energy comparable to what the Sun releases in its entire lifetime. The field of GRBs has developed rapidly and matured over the past decades. Written by a leading researcher, this text presents a thorough treatment of every aspect of the physics of GRBs. It starts with an overview of the field and an introduction to GRB phenomenology. After laying out the basics of relativity, relativistic shocks, and leptonic and hadronic radiation processes, the volume covers all topics related to GRBs, including a general theoretical framework, afterglow and prompt emission models, progenitor, central engine, multi-messenger aspects (cosmic rays, neutrinos, and gravitational waves), cosmological connections, and broader impacts on fundamental physics and astrobiology. It is suitable for advanced undergraduates, graduate students, and experienced researchers in the field of GRBs and high-energy astrophysics in general.

This book provides a comprehensive introduction to photoelectron angular distributions and their use in the laboratory to study light-matter interactions. Photoelectron angular distribution measurements are useful because they can shed light on atomic and molecular electronic configurations and system dynamics, as well as provide information about quantum transition amplitudes and relative phases that are not obtainable from other types of measurements. For example, recent measurements of molecular-frame photoelectron angular distributions have been used to extract photoelectron emission delays in the attosecond range which can provide ultra-sensitive maps of molecular potentials. Additionally, photoelectron angular distribution measurements are an essential tool for studying negative ions. Here, the author presents a detailed, yet easily accessible, theoretical background necessary for experimentalists performing photoelectron angular distribution measurements to better understand their results. The various physical influences on photoelectron angular distributions are revealed through analytical models with the use of angular momentum coupling algebra and spherical tensor operators. The classical and quantum treatments of photoelectron angular distributions are covered clearly and systematically, and the book includes, as well, a chapter on relativistic interactions. Furthermore, the primary methods used to measure photoelectron angular distributions in the laboratory, such as photodetachment electron spectroscopy, velocity-map imaging, and cold target recoil ion momentum spectroscopy, are described. This book features introductory material as well as new insights on the topic, such as the use of angular momentum transfer theory to understand the process of photoelectron detachment in atoms and molecules. Including key derivations, worked examples, and additional exercises for readers to try on their own, this book serves as both a critical guide for young researchers entering the field and as a useful reference for experienced practitioners.

An up-to-date text, covering the concept of incomplete fusion (ICF) in heavy ion (HI) interactions at energies below 10 MeV/ nucleon. Important concepts including the exciton model, the Harp Miller and Berne model, Hybrid model, Sum rule model, Hot spot model and promptly emitted particles model are covered in depth. It studies the ICF and PE-emission in heavy ion reactions at low energies using off-beam and in-beam experimental techniques. Theories of complete fusion (CF) of heavy ions based on Compound Nucleus (CN) mechanism of statistical nuclear reactions, details of the Computer code PACE4 based on CN mechanism, pre-equilibrium (PE) emission, modeling of (ICF) and their limits of application are discussed in detail.